〜際(さい)
When/at the time of/on the occasion of (formal)
About
~際 can attach to a present/past casual verb, or a noun using の, and is used to express "when" or "on the occasion of".
~際 is most commonly used in polite/formal spoken situations, or in written contexts.
〜際 may appear on its own (written), or with は, に, or には attached. It may also attach to a following noun using の.
〜際 has a nuance of officiality to it, and isn't natural to use with unimportant or mundane actions.
E.g. 免許証を更新する際に、こちらの書類をお持ちください。 "When renewing your license, please bring these forms."
E.g. お帰りの際は、お忘れ物にご注意ください。 "When leaving, please be sure not to forget any belongings."
The phrase,「この際」 means something like "since we have a chance..." or "now is a good time to do..." (lit. "this opportunity"), and is used much more colloquially than 際 typically is:
E.g. この際、余っている野菜は全部入れちゃおうよ。 "We may as well put in all of the leftover veggies."
E.g. この際だからはっきり言うけど、部屋の掃除をして。 "I'll take this occasion to say it clearly: clean your room."

~際 is used to express "when" or "on the occasion of"

~際 is most commonly used in polite/formal spoken situations, or in written contexts
Summary
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